分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： On-chip efficient nonlinear functions are instrumental in escalating the utilities and performance of photonic integrated circuits (PICs), especially for a wide range of classical and quantum applications, such as tunable coherent radiation, optical frequency conversion, spectroscopy, quantum science, etc. Lithium tantalate (LT) has been widely used in nonlinear wavelength converters, surface acoustic wave resonators, and electro-optic, acoustic-optic devices owing to its excellent optical properties. Here, we fabricated a Z-cut lithium tantalate on insulator (LTOI) microdisk with high quality(Q) factors in both telecom (10$^{6}$) and visible (10$^{5}$) bands by optimizing the fabrication. With the Q factor of the LTOI microdisk increasing, we can obtain higher pump light intensity in the cavity which is beneficial to get more optical nonlinear effect easily. By making use of the mode phase matching of interacting waves and inputting high pump power, we experimentally observed on-chip near-infrared light, visible (red, green), and ultraviolet (UV) from microresonator-based $ \chi^{(2)}-\chi^{(2)}$, $ \chi^{(2)}-\chi^{(3)}$, and $\chi^{(2)}$ nonlinear processes such as cascaded four-wave mixing (cFWM), cascaded sum-frequency generation (cSFG), third harmonic generation (THG), second harmonic generation (SHG). It is believed that the LTOI can support a variety of on-chip optical nonlinear processes, which heralds its new application potential in integrated nonlinear photonics.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： Due to their capacity for non-classical light generation, high-efficiency second-order nonlinear parametric processes play an important role in quantum photonic technology, and chip-scale realization of these processes is recognized as the key to building efficient light sources for integrated quantum photonic circuits. To achieve ultra-high nonlinear conversion efficiency, traditional method uses quasi-phase matching (QPM) technology. However, QPM requires electric field poling, which is incompatible with the CMOS fabrication process, and this hinders the wafer-scale production of integrated photonic circuits. In this paper, we demonstrate efficient spontaneous quasi-phase matched (SQPM) frequency conversion in a micro-racetrack resonator. Our approach does not involve poling, but exploits the anisotropy of the ferroelectric crystals to allow the phase-matching condition to be fulfilled spontaneously as the TE-polarized light circulates in a specifically designed racetrack resonator. SQPM second harmonic generation is observed with a normalized intracavity conversion efficiency of 0.85%/W, corresponding to the 111st-order QPM. This could theoretically reach 186,000%/W by first-order QPM. In this case such high intracavity conversion efficiency can be implemented in practice with an optimized outward coupling. Our configurable SQPM approach will benefit the application of nonlinear frequency conversion in chip-scale integrated photonics with CMOS-compatible fabrication processes, and is applicable to other on-chip nonlinear processes such as quantum frequency conversion or frequency-comb generation.
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